Optical Nanoimaging for Block Copolymer Self-Assembly.

One approach toward optical nanoimaging involves sequential molecular localization of photoswitchable fluorophores to achieve high resolution beyond optical limit of diffraction. Block copolymer micelles assembled from polystryrene-block-poly(ethylene oxide) block copolymers (PSt-b-PEO) are visualiz...

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Publicado en:Journal of the American Chemical Society Vol. 137; no. 7; pp. 2436 - 2440
Autores principales: Jie Yan, Ling-Xi Zhao, Chong Li, Zhe Hu, Guo-Feng Zhang, Ze-Qiang Chen, Tao Chen, Zhen-Li Huang, Jintao Zhu, Ming-Qiang Zhu
Formato: Artículo
Publicado: American Chemical Society 2/25/2015
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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        10.1021/ja512189a
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        atl: Optical Nanoimaging for Block Copolymer Self-Assembly.
      aug:
        au:
          Jie Yan
          Ling-Xi Zhao
          Chong Li
          Zhe Hu
          Guo-Feng Zhang
          Ze-Qiang Chen
          Tao Chen
          Zhen-Li Huang
          Jintao Zhu
          Ming-Qiang Zhu
        affil:
          Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan, Hubei 430074, China
          College of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, Hubei 430074, China
      su:
        Chromophores
        Epoxy compounds
        Copolymer micelles
        Block copolymers
        Electromagnetic waves
      sug:
        subj:
          Chromophores
          Epoxy compounds
          Copolymer micelles
          Block copolymers
          Electromagnetic waves
      ab: One approach toward optical nanoimaging involves sequential molecular localization of photoswitchable fluorophores to achieve high resolution beyond optical limit of diffraction. Block copolymer micelles assembled from polystryrene-block-poly(ethylene oxide) block copolymers (PSt-b-PEO) are visualized in optical nanoimaging by staining the polystyrene blocks with spiropyrans (SPs). SPs localized in hydrophobic phase of block copolymer micelles exhibit reversible fluorescence on-off switching at alternating irradiation of UV and visible light. Phase-selective distribution of SPs in block copolymer micelles enables optical nanoimaging of microphase structures of block copolymer self-assembly at 50-nm resolution. To date, this is the sturdiest realization of optical nanoimaging with subdiffraction resolution for solution self-assembly of block copolymers.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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