Dual Element Intercalation into 2D Layered BiSe Nanoribbons.

We demonstrate the intercalation of multiple zero-valent atomic species into two-dimensional (2D) layered BiSe nanoribbons. Intercalation is performed chemically through a stepwise combination of disproportionation redox reactions, hydrazine reduction, or carbonyl decomposition. Traditional intercal...

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Publicado en:Journal of the American Chemical Society Vol. 137; no. 16; pp. 5431 - 5438
Autores principales: Chen, Karen P., Chung, Frank R., Mengjing Wang, Koski, Kristie J.
Formato: Artículo
Publicado: American Chemical Society 4/29/2015
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      dt: 4/29/2015
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      pub: American Chemical Society
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        10.1021/jacs.5b00666
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        atl: Dual Element Intercalation into 2D Layered BiSe Nanoribbons.
      aug:
        au:
          Chen, Karen P.
          Chung, Frank R.
          Mengjing Wang
          Koski, Kristie J.
        affil: Department of Chemistry, Brown University, 324 Brook St. Box H, Providence Rhode Island 02912, United States
      su:
        Nanoribbons
        Nanobelts
        Chemical reactions
        Carbonyl compounds
        Atoms
      sug:
        subj:
          Nanoribbons
          Nanobelts
          Chemical reactions
          Carbonyl compounds
          Atoms
      ab: We demonstrate the intercalation of multiple zero-valent atomic species into two-dimensional (2D) layered BiSe nanoribbons. Intercalation is performed chemically through a stepwise combination of disproportionation redox reactions, hydrazine reduction, or carbonyl decomposition. Traditional intercalation is electrochemical thus limiting intercalant guests to a single atomic species. We show that multiple zero-valent atoms can be intercalated through this chemical route into the host lattice of a 2D crystal. Intermetallic species exhibit unique structural ordering demonstrated in a variety of superlattice diffraction patterns. We believe this method is general and can be used to achieve a wide variety of new 2D materials previously inaccessible.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2015
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