Synthesis and use of [Cd(Detu)₂(OOCCH₃)₂]·H₂O as single molecule precursor for Cds nanoparticles.

Substituted thiourea ligands are of interest because they possess various donor sites for metal ions and their application in separation of metal ions and as antimicrobial agents. The coordination of the sulfur donor atom led to interest in them as precursor for semiconductor nanoparticles. In this...

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Publicado en:Scientific World Journal pp. 907562 - 907563
Autor principal: Ajibade, Peter A
Formato: research Journal Article
Publicado: Wiley-Blackwell 2013
Acceso en línea:Ver este registro en EBSCOhost
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      jtl: Scientific World Journal
      issn: 1537744X
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      dt: 2013
      pid: 480
      pub: Wiley-Blackwell
      place: Malden, Massachusetts
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        10.1155/2013/907562
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        104121159
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        atl: Synthesis and use of [Cd(Detu)₂(OOCCH₃)₂]·H₂O as single molecule precursor for Cds nanoparticles.
      aug:
        au: Ajibade, Peter A
        affil: Department of Chemistry, University of Fort Hare, Private Bag X1314, Alice 5700, South Africa.
      sug:
        subj:
          Cadmium Compounds
          Metals
          Sulfides
          Chemistry
          Chemistry, Physical
          Microscopy, Electron, Scanning
          Microscopy, Electron
          Molecular Structure
          Spectrophotometry, Infrared
          Chemistry, Analytical
      ab: Substituted thiourea ligands are of interest because they possess various donor sites for metal ions and their application in separation of metal ions and as antimicrobial agents. The coordination of the sulfur donor atom led to interest in them as precursor for semiconductor nanoparticles. In this study, cadmium(II) complex of diethylthiourea was synthesized and characterized by elemental analysis, FTIR, and X-ray crystallography. Single crystal X-ray structure of the complex showed that the octahedral geometry around the Cd ion consists of two molecules of diethylthiourea acting as monodentate ligands and two chelating acetate ions. The thermal decomposition of the compound showed that it decomposed to give CdS. The compound was thermolysed in hexadecylamine (HDA) to prepare HDA-capped CdS nanoparticles. The absorption spectrum showed blue shifts in its absorption band edges which clearly indicated quantum confinement effect, and the emission spectrum showed characteristic band edge luminescence. The broad diffraction peaks of the XRD pattern showed the materials to be of the nanometric size.
      pubtype: Academic Journal
      doctype:
        research
        Journal Article
      ougenre: Article
    language: English
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