Characterization of phthalate exposure among pregnant women assessed by repeat air and urine samples.

BACKGROUND: Although urinary concentrations of phthalate metabolites are frequently used as biomarkers in epidemiologic studies, variability during pregnancy has not been characterized. METHODS: We measured phthalate metabolite concentrations in spot urine samples collected from 246 pregnant Dominic...

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Publicado en:Environmental Health Perspectives Vol. 116; no. 4; pp. 467 - 474
Autores principales: Adibi JJ, Whyatt RM, Williams PL, Calafat AM, Camann D, Herrick R, Nelson H, Bhat HK, Perera FP, Silva MJ, Hauser R
Formato: research tables/charts Journal Article
Publicado: National Institute of Environmental Health Sciences Apr2008
Acceso en línea:Ver este registro en EBSCOhost
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      dt: Apr2008
      vid: 116
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      pub: National Institute of Environmental Health Sciences
      place: Research Triangle Park, North Carolina
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        2009892216
        10.1289/ehp.10749
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        atl: Characterization of phthalate exposure among pregnant women assessed by repeat air and urine samples.
      aug:
        au:
          Adibi JJ
          Whyatt RM
          Williams PL
          Calafat AM
          Camann D
          Herrick R
          Nelson H
          Bhat HK
          Perera FP
          Silva MJ
          Hauser R
        affil: Department of Environmental Health, Harvard School of Public Health, Boston, Massachusetts, USA
      sug:
        subj:
          Air Pollution, Indoor
          Carboxylic Acids Urine
          Confidence Intervals
          Female
          Funding Source
          Infant, Newborn
          Intraclass Correlation Coefficient
          New York
          Pregnancy
          Repeated Measures
          Sensitivity and Specificity
          Human
          Infant, Newborn: birth-1 month
          Female
      ab: BACKGROUND: Although urinary concentrations of phthalate metabolites are frequently used as biomarkers in epidemiologic studies, variability during pregnancy has not been characterized. METHODS: We measured phthalate metabolite concentrations in spot urine samples collected from 246 pregnant Dominican and African-American women. Twenty-eight women had repeat urine samples collected over a 6-week period. We also analyzed 48-hr personal air samples (n = 96 women) and repeated indoor air samples (n = 32 homes) for five phthalate diesters. Mixed-effects models were fit to evaluate reproducibility via intraclass correlation coefficients (ICC). We evaluated the sensitivity and specificity of using a single specimen versus repeat samples to classify a woman's exposure in the low or high category. RESULTS: Phthalates were detected in 85-100% of air and urine samples. ICCs for the unadjusted urinary metabolite concentrations ranged from 0.30 for mono-ethyl phthalate to 0.66 for monobenzyl phthalate. For indoor air, ICCs ranged from 0.48 [di-2-ethylhexyl phthalate (DEHP)] to 0.83 [butylbenzyl phthalate (BBzP)]. Air levels of phthalate diesters correlated with their respective urinary metabolite concentrations for BBzP (r = 0.71), di-isobutyl phthalate (r = 0.44), and diethyl phthalate (DEP; r = 0.39). In women sampled late in pregnancy, specific gravity appeared to be more effective than creatinine in adjusting for urine dilution. CONCLUSIONS: Urinary concentrations of DEP and DEHP metabolites in pregnant women showed lower reproducibility than metabolites for di-n-butyl phthalate and BBzP. A single indoor air sample may be sufficient to characterize phthalate exposure in the home, whereas urinary phthalate biomarkers should be sampled longitudinally during pregnancy to minimize exposure misclassification.
      pubtype: Academic Journal
      doctype:
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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