Application of Molecular Modeling to Development of New Factor Xa Inhibitors.

In consequence of the key role of factor Xa in the clotting cascade and absence of its activity in the processes that do not affect coagulation, this protein is an attractive target for development of new blood coagulation inhibitors. Factor Xa is more effective and convenient target for creation of...

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Published in:BioMed Research International Vol. 2015; pp. 1 - 16
Main Authors: Sulimov, Vladimir B., Gribkova, Irina V., Kochugaeva, Maria P., Katkova, Ekaterina V., Sulimov, Alexey V., Kutov, Danil C., Shikhaliev, Khidmet S., Medvedeva, Svetlana M., Krysin, Michael Yu., Sinauridze, Elena I., Ataullakhanov, Fazoil I.
Format: equations & formulas pictorial research tables/charts Journal Article
Published: Wiley-Blackwell 9/21/2015
Online Access:View this record in EBSCOhost
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      dt: 9/21/2015
      vid: 2015
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      pub: Wiley-Blackwell
      place: Malden, Massachusetts
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        10.1155/2015/120802
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        atl: Application of Molecular Modeling to Development of New Factor Xa Inhibitors.
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        au:
          Sulimov, Vladimir B.
          Gribkova, Irina V.
          Kochugaeva, Maria P.
          Katkova, Ekaterina V.
          Sulimov, Alexey V.
          Kutov, Danil C.
          Shikhaliev, Khidmet S.
          Medvedeva, Svetlana M.
          Krysin, Michael Yu.
          Sinauridze, Elena I.
          Ataullakhanov, Fazoil I.
        affil: Research Computer Center, Moscow State University, Leninskie Gory 1, Building 4, Moscow 119991, Russia
      sug:
        subj:
          Models, Biological
          Blood Coagulation Factors
          Enzyme Inhibitors
          Molecular Structure
          Proteins
          In Vitro Studies
          Binding Sites
          Descriptive Statistics
          Data Analysis Software
          Odds Ratio
          Confidence Intervals
          Cell Line
          Biochemistry
          Funding Source
      ab: In consequence of the key role of factor Xa in the clotting cascade and absence of its activity in the processes that do not affect coagulation, this protein is an attractive target for development of new blood coagulation inhibitors. Factor Xa is more effective and convenient target for creation of anticoagulants than thrombin, inhibition of which may cause some side effects. This study is aimed at finding new inhibitors of factor Xa by molecular computer modeling including docking SOL and postdocking optimization DISCORE programs. After validation of molecular modeling methods on well-known factor Xa inhibitors the virtual screening of NCI Diversity and Voronezh State University databases of ready-made low molecular weight species has been carried out. Seventeen compounds selected on the basis of modeling results have been tested experimentally in vitro. It has been found that 12 of them showed activity against factor Xa (IC50 = 1.8-40 μM). Based on analysis of the results, the new original compound was synthesized and experimentally verified. It shows activity against factor Xa with IC50 value of 0.7 μM.
      pubtype: Academic Journal
      doctype:
        equations & formulas
        pictorial
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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