Al[18F]NOTA-T140 Peptide for Noninvasive Visualization of CXCR4 Expression.

Purpose: Chemokine receptor CXCR4 plays an important role in tumor aggressiveness, invasiveness, and metastasis formation. Quantification of CXCR4 expression by tumors may have an impact on prediction and evaluation of tumor response to therapies. In this study, we developed a robust and straightfor...

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Publicado en:Molecular Imaging & Biology Vol. 18; no. 1; pp. 135 - 143
Autores principales: Yan, Xuefeng, Niu, Gang, Wang, Zhe, Yang, Xiangyu, Kiesewetter, Dale, Jacobson, Orit, Shen, Baozhong, Chen, Xiaoyuan, Kiesewetter, Dale O
Formato: research Journal Article
Publicado: Springer Nature Feb2016
Acceso en línea:Ver este registro en EBSCOhost
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      dt: Feb2016
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      pub: Springer Nature
      place: New York, New York
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        10.1007/s11307-015-0872-2
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        atl: Al[18F]NOTA-T140 Peptide for Noninvasive Visualization of CXCR4 Expression.
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          Yan, Xuefeng
          Niu, Gang
          Wang, Zhe
          Yang, Xiangyu
          Kiesewetter, Dale
          Jacobson, Orit
          Shen, Baozhong
          Chen, Xiaoyuan
          Kiesewetter, Dale O
        affil: Laboratory of Molecular Imaging and Nanomedicine (LOMIN), National Institute of Biomedical Imaging and Bioengineering (NIBIB), National Institutes of Health (NIH), Bethesda USA
      sug:
        subj:
          Fluorine Radioisotopes Metabolism
          Receptors, Cell Surface Metabolism
          Aluminum Metabolism
          Oligopeptides Metabolism
          Heterocyclic Compounds Metabolism
          Hamsters
          Animal Studies
          Oligopeptides
          Cytokines Metabolism
          Rodents
          Mice
          Neoplasm Metastasis
          Heterocyclic Compounds
          Tomography, Emission-Computed
          Binding Sites
          Funding Source
      ab: Purpose: Chemokine receptor CXCR4 plays an important role in tumor aggressiveness, invasiveness, and metastasis formation. Quantification of CXCR4 expression by tumors may have an impact on prediction and evaluation of tumor response to therapies. In this study, we developed a robust and straightforward F-18 labeling route of T140, a CXCR4 peptide-based antagonist.Procedures: T140 derivative was conjugated to 1,4,7-triazacyclononane-triacetic acid (NOTA) and labeled with Al[(18)F]. Al[(18)F]NOTA-T140 was evaluated in vitro in cell-based assay and stability in mouse serum and in vivo using CXCR4 positive and negative tumor xenograft models.Results: Labeling of Al[(18)F]NOTA-T140 was completed within 30 min with a radiochemical yield of 58 ± 5.3 % at the end of synthesis, based on fluoride-18 activity. Al[(18)F]NOTA-T140 accumulated in CHO-CXCR4 positive but not negative tumors. Al[(18)F]NOTA-T140 uptake in the tumors correlated with CXCR4 protein expression. Moreover, Al[(18)F]NOTA-T140 had high accumulation in CXCR4-positive metastatic tumors.Conclusions: The simplicity of Al[(18)F]NOTA-T140 labeling along with its properties to specifically image CXCR4 expression by tumors warrant further clinical application for the diagnosis of CXCR4 clinically.
      pubtype: Academic Journal
      doctype:
        research
        Journal Article
      ougenre: Article
    language: English
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