Facile Synthesis of Photofunctional Nanolayer Coatings on Titanium Substrates.

We developed a two-step chemical bonding process using photosensitizer molecules to fabricate photofunctional nanolayer coatings on hematoporphyrin- (HP-) coated Ti substrates. In the first step, 3-aminopropyltriethoxysilane was covalently functionalized onto the surface of the Ti substrates to prov...

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Publicado en:BioMed Research International Vol. 2016; pp. 1 - 10
Autores principales: Choi, Kyong-Hoon, Kim, Jung-Gil, Kang, Byungman, Kim, Ho-Joong, Park, Bong Joo
Formato: pictorial research tables/charts Journal Article
Publicado: Wiley-Blackwell 3/24/2016
Acceso en línea:Ver este registro en EBSCOhost
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        23146133
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      issn: 23146133
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      dt: 3/24/2016
      vid: 2016
      pid: 480
      pub: Wiley-Blackwell
      place: Malden, Massachusetts
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        113954488
        113954488
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        10.1155/2016/4318917
        113954488
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        atl: Facile Synthesis of Photofunctional Nanolayer Coatings on Titanium Substrates.
      aug:
        au:
          Choi, Kyong-Hoon
          Kim, Jung-Gil
          Kang, Byungman
          Kim, Ho-Joong
          Park, Bong Joo
        affil: Plasma Bioscience Research Center, Kwangwoon University, 20 Kwangwoon-gil, Nowon-gu, Seoul 139-701, Republic of Korea
      sug:
        subj:
          Nanostructures
          Titanium
          Nanotechnology
          Prostheses and Implants
          Chemistry, Physical
          Porphyrins
          Silicon Compounds
          Spectrometry, X-Ray Emission
          Microscopy, Electron, Scanning
          Spectrophotometry Methods
          Heterocyclic Compounds
          Materials Testing
          Toxicity Tests
          Oxygen
          Cell Culture Techniques
          T-Tests
          P-Value
          Descriptive Statistics
          Animal Studies
          Mice
          Funding Source
      ab: We developed a two-step chemical bonding process using photosensitizer molecules to fabricate photofunctional nanolayer coatings on hematoporphyrin- (HP-) coated Ti substrates. In the first step, 3-aminopropyltriethoxysilane was covalently functionalized onto the surface of the Ti substrates to provide heterogeneous sites for immobilizing the HP molecules. Then, HP molecules with carboxyl groups were chemically attached to the amine-terminated nanolayer coatings via a carbodiimide coupling reaction. The microstructure and elemental and phase composition of the HP-coated Ti substrates were investigated using field-emission scanning electron microscopy and energy-dispersive X-ray spectrometry. The photophysical properties of the photofunctional nanolayer coatings were confirmed using reflectance ultraviolet-visible absorption and emission spectrophotometry. The singlet oxygen generation efficiency of the photofunctional nanolayer coatings was determined using the decomposition reaction of 1,3-diphenylisobenzofuran. The HP-coated Ti substrates exhibited good biocompatibility without any cytotoxicity, and these nanolayer coatings generated singlet oxygen, which can kill microorganisms using only visible light.
      pubtype: Academic Journal
      doctype:
        pictorial
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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