New-Structure-Type Fe-Based Superconductors: CaAFeAs (A = K, Rb, Cs) and SrAFeAs (A = Rb, Cs).

Fe-based superconductors have attracted research interest because of their rich structural variety, which is due to their layered crystal structures. Here we report the new-structure-type Fe-based superconductors CaAFe4As4 (A = K, Rb, Cs) and SrAFeAs (A = Rb, Cs), which can be regarded as hybrid pha...

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Publicado en:Journal of the American Chemical Society Vol. 138; no. 10; pp. 3410 - 3416
Autores principales: Akira Iyo, Kenji Kawashima, Tatsuya Kinjo, Taichiro Nishio, Shigeyuki Ishida, Hiroshi Fujihisa, Yoshito Gotoh, Kunihiro Kihou, Hiroshi Eisaki, Yoshiyuki Yoshida
Formato: Artículo
Publicado: American Chemical Society 3/16/2016
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Acceso en línea:Ver este registro en EBSCOhost
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      dt: 3/16/2016
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      pub: American Chemical Society
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        114330734
        10.1021/jacs.5b12571
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        atl: New-Structure-Type Fe-Based Superconductors: CaAFeAs (A = K, Rb, Cs) and SrAFeAs (A = Rb, Cs).
      aug:
        au:
          Akira Iyo
          Kenji Kawashima
          Tatsuya Kinjo
          Taichiro Nishio
          Shigeyuki Ishida
          Hiroshi Fujihisa
          Yoshito Gotoh
          Kunihiro Kihou
          Hiroshi Eisaki
          Yoshiyuki Yoshida
        affil:
          National Institute of Advanced Industrial Science and Technology (AIST), 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568, Japan
          IMRA Material R&D Co., Ltd., 2-1 Asahi-machi, Kariya, Aichi 448-0032, Japan
          Department of Physics, Tokyo University of Science, 1-3 Kagurazaka, Shinjuku, Tokyo 162-8601, Japan
      su:
        Superconductors
        Crystal structure
        Iron compounds
        Calcium compounds
        Solid solutions
        Crystallography
      sug:
        subj:
          Superconductors
          Crystal structure
          Iron compounds
          Calcium compounds
          Solid solutions
          Crystallography
      ab: Fe-based superconductors have attracted research interest because of their rich structural variety, which is due to their layered crystal structures. Here we report the new-structure-type Fe-based superconductors CaAFe4As4 (A = K, Rb, Cs) and SrAFeAs (A = Rb, Cs), which can be regarded as hybrid phases between AeFeAs (Ae = Ca, Sr) and AFeAs. Unlike solid solutions such as (Ba1-xKx)FeAs and (SrNa)FeAs, Ae and A do not occupy crystallographically equivalent sites because of the large differences between their ionic radii. Rather, the Ae and A layers are inserted alternately between the FeAs layers in the c-axis direction in AeAFeAs (AeA1144). The ordering of the Ae and A layers causes a change in the space group from I4/mmm to P4/mmm, which is clearly apparent in powder X-ray diffraction patterns. AeA1144 is the first known structure of this type among not only Fe-based superconductors but also other materials. AeA1144 is formed as a line compound, and therefore, each AeA1144 has its own superconducting transition temperature of approximately 31-36 K.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2016
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