Investigation of Molecular Structure, Chemical Reactivity and Stability for Pyrrole Substitutes (Dual Anchoring System) Using Density Functional Theory.

The theoretical electron properties of Pyrrole Substitutes (R1, R2, R3 and R4) were carried out by using quantum chemical calculations. The optimized structures were obtained by the Density Functional Theory DFT/B3LYP level of theory using the basis set 6-31G. The optimized structures of compounds h...

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Publicado en:Journal of Basrah Researches (Sciences) Vol. 41; no. 3A; pp. 24 - 36
Autores principales: Al-shawi, Jasim M., Hussain, Kawkab A., Ismael, Sadiq M-H.
Formato: Artículo
Publicado: Republic of Iraq Ministry of Higher Education & Scientific Research (MOHESR) 2015
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        atl: Investigation of Molecular Structure, Chemical Reactivity and Stability for Pyrrole Substitutes (Dual Anchoring System) Using Density Functional Theory.
      aug:
        au:
          Al-shawi, Jasim M.
          Hussain, Kawkab A.
          Ismael, Sadiq M-H.
        affil: Department of Chemistry -- College of Education for Pure Science University of Basrah -- Iraq
      su:
        Molecular structure
        Reactivity (Chemistry)
        Chemical stability
        Pyrroles
        Density functional theory
        Electrons
      sug:
        subj:
          Molecular structure
          Reactivity (Chemistry)
          Chemical stability
          Pyrroles
          Density functional theory
          Electrons
      keyword:
        Band Gap
        DFT/B3LYP
        Pyrrole Substitutes
        structural and electronic properties
        الخواص الالكترونية والتركيبية
        دالة الكثافة الالكترونية
        فجوة الطاقت
        معوضات البايرول
      ab: The theoretical electron properties of Pyrrole Substitutes (R1, R2, R3 and R4) were carried out by using quantum chemical calculations. The optimized structures were obtained by the Density Functional Theory DFT/B3LYP level of theory using the basis set 6-31G. The optimized structures of compounds have the global minimum energy. It was found that the dipole moment of compound (R1) have high values compared with the Compounds (R2,R3,R4). Global descriptors such as the MO energies of HOMO, LUMO levels and ΔE, were determined and used to identify the differences in the stability and reactivity of compounds. In general, the calculated values lead to the conclusion that on the one hand the stability of the compounds are R3>R4>R1>R2. On the other hand, the theoretical study of novel acceptor-donor organic materials based on these compounds has been investigated. Different electron side groups were introduced to investigate their effects on the electronic structure; HOMO, LUMO and energy gap. The structural and electronic study as shown in this paper in hand for these compounds could help to design more efficient functional photovoltaic organic materials.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2015
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