Treatment of chemical cleaning wastewater and cost optimization by response surface methodology coupled nonlinear programming.

The real alkaline cleaning wastewater (ACW) was treated by a process consisting of neutralization, NaClO oxidation and aluminum sulfate (AS) coagulation, and a novel response surface methodology coupled nonlinear programming (RSM-NLP) approach was developed and used to optimize the oxidation-coagula...

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Published in:Journal of Environmental Management Vol. 198; pp. 12 - 21
Main Authors: Yang, Yang, Zhou, Zhen, Lu, Chenjie, Chen, Yunke, Ge, Honghua, Wang, Libing, Cheng, Cheng
Format: Article
Published: Academic Press Inc. Aug2017 Part 2
Subjects:
Online Access:View this record in EBSCOhost
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        03014797
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      jtl: Journal of Environmental Management
      issn: 03014797
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      dt: Aug2017 Part 2
      vid: 198
      pid: 735
      pub: Academic Press Inc.
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        123269196
        10.1016/j.jenvman.2017.05.009
      ppf: 12
      ppct: 9
      formats:
      tig:
        atl: Treatment of chemical cleaning wastewater and cost optimization by response surface methodology coupled nonlinear programming.
      aug:
        au:
          Yang, Yang
          Zhou, Zhen
          Lu, Chenjie
          Chen, Yunke
          Ge, Honghua
          Wang, Libing
          Cheng, Cheng
        affil:
          College of Environmental and Chemical Engineering, Shanghai University of Electric Power, 2588 Changyang Road, Shanghai, 200090, China
          Shanghai Ahill Chemical Products Co., Ltd, 1038 Guoshun Road, Shanghai, 200090, China
      su:
        Wastewater treatment
        Chemical cleaning
        Coagulation (Sewage purification)
        Aluminum sulfate
        Nonlinear programming
        Response surfaces (Statistics)
      sug:
        subj:
          Other Basic Inorganic Chemical Manufacturing
          All other basic inorganic chemical manufacturing
          Sewage Treatment Facilities
          Wastewater treatment
          Chemical cleaning
          Coagulation (Sewage purification)
          Aluminum sulfate
          Nonlinear programming
          Response surfaces (Statistics)
      keyword:
        Cleaning wastewater
        Coagulation
        NaClO oxidation
        Neutralization
        Response surface methodology
        Cleaning wastewater
        Coagulation
        NaClO oxidation
        Neutralization
        Response surface methodology
      ab: The real alkaline cleaning wastewater (ACW) was treated by a process consisting of neutralization, NaClO oxidation and aluminum sulfate (AS) coagulation, and a novel response surface methodology coupled nonlinear programming (RSM-NLP) approach was developed and used to optimize the oxidation-coagulation process under constraints of relevant discharge standards. Sulfuric acid neutralization effectively removed chemical oxygen demand (COD), surfactant alkylphenol ethoxylates (OP-10) and silicate at the optimum pH of 7.0, with efficiencies of 62.3%, >82.7% and 94.2%, respectively. Coagulation and adsorption by colloidal hydrated silica formed during neutralization were the major removal mechanisms. NaClO oxidation achieved almost complete removal of COD, but was ineffective for the removal of surfactant OP-10. AS coagulation followed by oxidation can efficiently remove OP-10 with the formation of Si-O-Al compounds. The optimum conditions for COD ≤100 mg/L were obtained at hypochlorite to COD molar ratio of 2.25, pH of 10.0 and AS dosage of 0.65 g Al/L, with minimum cost of 9.58 $/m 3 ACW. This study shows that the integrative RSM-NLP approach could effectively optimize the oxidation-coagulation process, and is attractive for techno-economic optimization of systems with multiple factors and threshold requirements for response variables.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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