Single Mo Atom Supported on Defective Boron Nitride Monolayer as an Efficient Electrocatalyst for Nitrogen Fixation: A Computational Study.

The production of ammonia (NH) from molecular dinitrogen (N) under mild conditions is one of the most attractive and challenging processes in chemistry. Here by means of density functional theory (DFT) computations, we systematically investigated the potential of single transition metal atoms (Sc to...

Descripción completa

Detalles Bibliográficos
Publicado en:Journal of the American Chemical Society Vol. 139; no. 36; pp. 12480 - 12488
Autores principales: Jingxiang Zhao, Zhongfang Chen
Formato: Artículo
Publicado: American Chemical Society 9/13/2017
Materias:
Acceso en línea:Ver este registro en EBSCOhost
fields @attributes:
  recordID: 1
pdfLink:
plink: https://search.ebscohost.com/login.aspx?direct=true&db=hlh&AN=125155154&site=ehost-live
header:
  @attributes:
    shortDbName: hlh
    uiTerm: 125155154
    longDbName: Humanities International Complete
    uiTag: AN
  controlInfo:
    bkinfo:
    jinfo:
      jid:
        00027863
        ACS
      jtl: Journal of the American Chemical Society
      issn: 00027863
      maglogo: N
    pubinfo:
      dt: 9/13/2017
      vid: 139
      iid: 36
      pid: 997
      pub: American Chemical Society
    artinfo:
      ui:
        125155154
        10.1021/jacs.7b05213
      ppf: 12480
      ppct: 8
      formats:
      tig:
        atl: Single Mo Atom Supported on Defective Boron Nitride Monolayer as an Efficient Electrocatalyst for Nitrogen Fixation: A Computational Study.
      aug:
        au:
          Jingxiang Zhao
          Zhongfang Chen
        affil:
          Key Laboratory of Photonic and Electronic Bandgap Materials, Ministry of Education, and College of Chemistry and Chemical Engineering, Harbin Normal University, Harbin, 150025, China
          Department of Chemistry, University of Puerto Rico, Rio Piedras Campus, San Juan, PR 00931, United States
      su:
        Boron nitride
        Nitrides
        Dinitrogenase reductase
        Density functional theory
        Molecular theory
      sug:
        subj:
          Boron nitride
          Nitrides
          Dinitrogenase reductase
          Density functional theory
          Molecular theory
      ab: The production of ammonia (NH) from molecular dinitrogen (N) under mild conditions is one of the most attractive and challenging processes in chemistry. Here by means of density functional theory (DFT) computations, we systematically investigated the potential of single transition metal atoms (Sc to Zn, Mo, Ru, Rh, Pd, and Ag) supported on the experimentally available defective boron nitride (TM-BN) monolayer with a boron monovacancy as a N fixation electrocatalyst. Our computations revealed that the single Mo atom supported by a defective BN nanosheet exhibits the highest catalytic activity for N fixation at room temperature through an enzymatic mechanism with a quite low overpotential of 0.19 V. The high spin-polarization, selective stabilization of NH* species, or destabilizing NH* species are responsible for the high activity of the Mo-embedded BN nanosheet for N fixation. This finding opens a new avenue of NH production by single-atom electrocatalysts under ambient conditions.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
    refInfo:
    copyright:
      @attributes:
        flag: Y
      dt:
        @attributes:
          year: 2017
    holdings:
      @attributes:
        islocal: N