DFT Studies of Graphene-Functionalised Derivatives of Capecitabine.

Cancer is one of the major problems for so many people around the world; therefore, dedicating efforts to explore efficient therapeutic methodologies is very important for researchers of life sciences. In this case, nanostructures are expected to be carriers of medicinal compounds for targeted drug...

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Publicado en:Zeitschrift für Naturforschung Section A: A Journal of Physical Sciences Vol. 72; no. 12; pp. 1131 - 1139
Autores principales: Aramideh, Mehdi, Mirzaei, Mahmoud, Khodarahmi, Ghadamali, Gülseren, Oğuz
Formato: Artículo
Publicado: De Gruyter Dec2017
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      dt: Dec2017
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        atl: DFT Studies of Graphene-Functionalised Derivatives of Capecitabine.
      aug:
        au:
          Aramideh, Mehdi
          Mirzaei, Mahmoud
          Khodarahmi, Ghadamali
          Gülseren, Oğuz
        affil:
          Department of Medicinal Chemistry, School of Pharmacy and Pharmaceutical Sciences, Isfahan University of Medical Sciences, Isfahan, Iran
          Department of Physics, Faculty of Science, Bilkent University, Ankara, Turkey
      su:
        Cancer treatment
        Density functional theory
        Graphene
        Targeted drug delivery
        Charge exchange
      sug:
        subj:
          Cancer treatment
          Density functional theory
          Graphene
          Targeted drug delivery
          Charge exchange
      keyword:
        Capecitabine
        Density Functional Theory
        Functionalisation
      ab: Cancer is one of the major problems for so many people around the world; therefore, dedicating efforts to explore efficient therapeutic methodologies is very important for researchers of life sciences. In this case, nanostructures are expected to be carriers of medicinal compounds for targeted drug design and delivery purposes. Within this work, the graphene (Gr)-functionalised derivatives of capecitabine (CAP), as a representative anticancer, have been studied based on density functional theory calculations. Two different sizes of Gr molecular models have been used for the functionalisation of CAP counterparts, CAP-Gr3 and CAP-Gr5, to explore the effects of Gr-functionalisation on the original properties of CAP. All singular and functionalised molecular models have been optimised and the molecular and atomic scale properties have been evaluated for the optimised structures. Higher formation favourability has been obtained for CAP-Gr5 in comparison with CAP-Gr3 and better structural stability has been obtained in the water-solvated system than the isolated gas-phase system for all models. The CAP-Gr5 model could play a better role of electron transferring in comparison with the CAP-Gr3 model. As a concluding remark, the molecular properties of CAP changed from singular to functionalised models whereas the atomic properties remained almost unchanged, which is expected for a carrier not to use significant perturbations to the original properties of the carried counterpart.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2017
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