Anti-Helicobacter pylori metabolites from Heterotheca inuloides (Mexican arnica).

Preparations of the plant known as “Mexican arnica” ( Heterotheca inuloides ) have been traditionally used for the treatment of several ailments including stomach ulcers and for relief of colic. To find possible biologically active components against these ailments, we tested the acetone extract as...

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Publicado en:Fitoterapia Vol. 127; pp. 314 - 322
Autores principales: Egas, Verónica, Salazar-Cervantes, Gabriela, Romero, Irma, Méndez-Cuesta, Carlos A., Rodríguez-Chávez, José Luis, Delgado, Guillermo
Formato: research Journal Article
Publicado: Elsevier B.V. Jun2018
Acceso en línea:Ver este registro en EBSCOhost
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      dt: Jun2018
      vid: 127
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      pub: Elsevier B.V.
      place: New York, New York
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        129847204
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        10.1016/j.fitote.2018.03.001
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        atl: Anti-Helicobacter pylori metabolites from Heterotheca inuloides (Mexican arnica).
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        au:
          Egas, Verónica
          Salazar-Cervantes, Gabriela
          Romero, Irma
          Méndez-Cuesta, Carlos A.
          Rodríguez-Chávez, José Luis
          Delgado, Guillermo
        affil: Instituto de Química, Universidad Nacional Autónoma de México, Circuito Exterior, Ciudad Universitaria, Coyoacán 04510, Mexico City, Mexico
      sug:
        subj:
          Plant Extracts Pharmacodynamics
          Helicobacter Infections Drug Therapy
          Helicobacter Pylori
          Terpenes
          Treatment Outcomes
          Spectrum Analysis
          Phytosterols
      ab: Preparations of the plant known as “Mexican arnica” ( Heterotheca inuloides ) have been traditionally used for the treatment of several ailments including stomach ulcers and for relief of colic. To find possible biologically active components against these ailments, we tested the acetone extract as well as different metabolites biosynthesized by this species, including cadinane-type sesquiterpenoids, triterpenes, phytosterols and flavonoids, against Helicobacter pylori . Among these compounds, sesquiterpenes 7-hydroxy-3,4-dihydrocadalene ( 3 ) and 7-hydroxy-cadalene ( 4 ) exhibited strong anti- H. pylori activity with MICs values of 1.95 and 3.91 μg/mL, respectively. HPLC-UV/DAD analyses revealed that both substances together with related compounds 7 , 8 and 9 were the major constituents of the acetone extract. Enzymatic assays and docking studies showed that unlike quercetin ( 10 ), a secondary metabolite also isolated from this species, compounds 3 and 4 did not inhibit the activity of urease, a potent virulence factor of H. pylori . Additionally, two new C 1 -C 9 secocadinanes ( 1 and 2 ) were isolated from the aerial parts of this species. Their structures were determined by extensive NMR and HRESIMS spectroscopic data analyses.
      pubtype: Academic Journal
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        research
        Journal Article
      ougenre: Article
    language: English
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