DFT Studies of Single Lithium Adsorption on Coronene.

Density functional theory (DFT) calculations were performed to study the adsorption of neutral and cationic forms of single lithium (Li) on representative original and each of oxygen/sulfur-terminated coronene monolayer surfaces. First, the monolayers of coronene structures were prepared. Next, Li/L...

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Publicado en:Zeitschrift für Naturforschung Section A: A Journal of Physical Sciences Vol. 73; no. 8; pp. 685 - 692
Autores principales: Harismah, Kun, Mirzaei, Mahmoud, Moradi, Reza
Formato: Artículo
Publicado: De Gruyter Aug2018
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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        atl: DFT Studies of Single Lithium Adsorption on Coronene.
      aug:
        au:
          Harismah, Kun
          Mirzaei, Mahmoud
          Moradi, Reza
        affil:
          Department of Chemical Engineering, Faculty of Engineering, Universitas Muhammadiyah Surakarta, Surakarta, Indonesia
          Bioinformatics Research Center, School of Pharmacy and Pharmaceutical Sciences, Isfahan University of Medical Sciences, Isfahan, Iran, Fax: +98 31 36680011
          Young Researchers and Elite Club, Arak Branch, Islamic Azad University, Arak, Iran
      su:
        Lithium
        Adsorption (Chemistry)
        Polycyclic aromatic compounds
        Density functional theory
        Molecular orbitals
      sug:
        subj:
          Lithium
          Adsorption (Chemistry)
          Polycyclic aromatic compounds
          Density functional theory
          Molecular orbitals
      keyword:
        Adsorption
        Coronene
        Density Functional Theory
      ab: Density functional theory (DFT) calculations were performed to study the adsorption of neutral and cationic forms of single lithium (Li) on representative original and each of oxygen/sulfur-terminated coronene monolayer surfaces. First, the monolayers of coronene structures were prepared. Next, Li/Li adsorptions were investigated on the surfaces of the already optimised coronene models. The results indicate that the singular coronene models can be considered as appropriate surfaces for Li/Li adsorption, with stronger Li adsorption. Localisations of LI/Li species were carefully examined at the central carbon zone of the monolayer surface; however, only one model showed discrepancy by getting localised at the monolayer edge. Energy levels and distribution patters for the molecular orbitals indicate the effects of atomic terminations and Li/Li adsorptions, in which the singular and Li-adsorbed models reveal identical results. Atomic-scale nuclear quadrupole resonance (NQR) properties were also evaluated, with the results indicating that the atomic properties can determine the major electronic properties for applying the coronene structure for specific applications.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2018
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