Urease and Carbonic Anhydrase Inhibitory Effect of Xanthones from Aspergillus nidulans , an Endophytic Fungus of Nyctanthes arbor-tristis.

Urease plays a major role in the pathogenesis of peptic and gastric ulcer and also causes acute pyelonephritis and development of infection-induced reactive arthritis. Carbonic anhydrases (CA) cause pathological disorders such as epilepsy (CA I), glaucoma, gastritis, renal, pancreatic carcinomas, an...

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Published in:Planta Medica Vol. 89; no. 4; pp. 377 - 385
Main Authors: Sana, Talea, Khan, Majid, Jabeen, Almas, Shams, Sidrah, Hadda, Taibi Ben, Begum, Sabira, Siddiqui, Bina Shaheen
Format: pictorial research tables/charts Journal Article
Published: Georg Thieme Verlag Stuttgart 2023
Online Access:View this record in EBSCOhost
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      jtl: Planta Medica
      issn: 00320943
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      dt: 2023
      vid: 89
      iid: 4
      pid: 4536
      pub: Georg Thieme Verlag Stuttgart
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        162801572
        162801572
        162801572
        10.1055/a-1908-0935
        162801572
      ppf: 377
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        atl: Urease and Carbonic Anhydrase Inhibitory Effect of Xanthones from Aspergillus nidulans , an Endophytic Fungus of Nyctanthes arbor-tristis.
      aug:
        au:
          Sana, Talea
          Khan, Majid
          Jabeen, Almas
          Shams, Sidrah
          Hadda, Taibi Ben
          Begum, Sabira
          Siddiqui, Bina Shaheen
        affil: H. E. J. Research Institute of Chemistry, International Center for Chemical and Biological Sciences, University of Karachi, Karachi, Pakistan
      sug:
        subj:
          Urease Metabolism
          Carbonic Anhydrase Inhibitors
          Heterocyclic Compounds Pharmacodynamics
          Fungi Metabolism
          Plant Extracts Pharmacodynamics
          Organic Chemicals Analysis
          Human
          Molecular Structure
          In Vitro Studies
          Plants
          Experimental Studies
          Molecular Docking Simulation
          Cytotoxicity Tests, Immunologic
          Funding Source
      ab: Urease plays a major role in the pathogenesis of peptic and gastric ulcer and also causes acute pyelonephritis and development of infection-induced reactive arthritis. Carbonic anhydrases (CA) cause pathological disorders such as epilepsy (CA I), glaucoma, gastritis, renal, pancreatic carcinomas, and malignant brain tumors (CA II). Although various synthetic urease and carbonic anhydrase inhibitors are known, these have many side effects. Hence, present studies were undertaken on ethyl acetate extract of Aspergillus nidulans , an endophytic fungus separated from the leaves of Nyctanthes arbor-tristis Linn. and led to the isolation of five furanoxanthones, sterigmatin (1), sterigmatocystin (3), dihydrosterigmatocystin (4), oxisterigmatocystin C (5), acyl-hemiacetal sterigmatocystin (6), and a pyranoxanthone (2). Acetylation of 3 gave compound O -acetyl sterigmatocystin (7). Their chemical structures were elucidated by1 H and13 C NMR and MS. The inhibitory effect of isolated compounds was evaluated on urease and carbonic anhydrase (b CA II) enzymes in vitro. Compounds 3 and 6 showed significant urease inhibition (IC50 19 and 21 µM), while other compounds exhibited varying degrees of urease inhibition (IC50 33 – 51 µM). Compounds 4, 6 and 7 exhibited significant inhibition of b CA II (IC50 values 21, 25 and 18 µM respectively), compounds 1 – 3 displayed moderate inhibition (IC50 61, 76 and 31 µM respectively) while 5 showed no inhibition. A mechanistic study of the most active urease inhibitors was also performed using enzyme kinetics and molecular docking. All compounds were found non-toxic on the NIH-3T3 cell line.
      pubtype: Periodical
      doctype:
        pictorial
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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