One-pot synthesis of nano-EMD for effective adsorption of toxic dyes.

A simple electrochemical technique was employed to synthesize nanocorn electrolytic manganese dioxide (MnO) (EMD) in the presence of the structure-directing agent poly(vinylpyrrolidone) (PVP) at the optimum concentration in an aqueous acidic manganese sulfate bath. X-ray diffraction and scanning ele...

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Publicado en:Transactions of the Charles S. Peirce Society Vol. 60; no. 1; pp. 166 - 178
Autores principales: Biswal, Avijit, Dhal, Jyoti Prakash, Das, Bijnyan Ranjan, Panda, Prasanna Kumar, Tripathy, Bankim Chandra
Formato: Artículo
Publicado: Indiana University Press Winter2024
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      dt: Winter2024
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        177680518
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        atl: One-pot synthesis of nano-EMD for effective adsorption of toxic dyes.
      aug:
        au:
          Biswal, Avijit
          Dhal, Jyoti Prakash
          Das, Bijnyan Ranjan
          Panda, Prasanna Kumar
          Tripathy, Bankim Chandra
        affil:
          Assistant Professor, Department of Chemistry, Odisha University of Technology and Research, Bhubaneswar, India
          Professor, Department of Chemistry, Odisha University of Technology and Research, Bhubaneswar, India
          PhD Research Scholar, Hydro and Electrometallurgy Department, CSIR–Institute of Minerals and Materials Technology, Bhubaneswar, India
          Chief Scientist, Hydro and Electrometallurgy Department, CSIR–Institute of Minerals and Materials Technology, Bhubaneswar, India
      su:
        Electrolytic manganese
        Malachite green
        Manganous sulfate
        Adsorption kinetics
        Dyes & dyeing
      sug:
        subj:
          Electrolytic manganese
          Malachite green
          Manganous sulfate
          Adsorption kinetics
          Dyes & dyeing
      keyword:
        adsorption
        Chicago sky blue
        electrodeposition
        EMD
        environmental impact
        hierarchical
        malachite green
        nanocorn
      ab: A simple electrochemical technique was employed to synthesize nanocorn electrolytic manganese dioxide (MnO) (EMD) in the presence of the structure-directing agent poly(vinylpyrrolidone) (PVP) at the optimum concentration in an aqueous acidic manganese sulfate bath. X-ray diffraction and scanning electron microscopy analyses confirmed the formation of γ-manganese dioxide with nanocorn-shaped crystals at the optimum concentration – namely, 20 mg/l PVP. The finely ground material was successfully employed in the removal of the toxic dyes Chicago sky blue (CSB) and malachite green (MG) from aqueous solution. Various process parameters such as different adsorbents, adsorbent dose, contact time, initial dye concentration and pH were varied and optimized for both dyes. It was found that EMD showed 99.61% adsorption efficiency at an optimum dose of 0.04 g/20 ml of the 100 mg/l CSB dye solution at room temperature within 20 min. However, the same EMD sample showed 99.5% adsorption efficiency at an optimum dose of 0.07 g/20 ml of the 100 mg/l MG dye solution at room temperature within 120 min. From the adsorption kinetics study, it was concluded that the adsorption process follows pseudo-second-order kinetics and the adsorption isotherm confirms that the reaction follows Langmuir adsorption for both dyes.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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      holder: Indiana University Press
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          year: 2024
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