Radical Hydroxyalkylation of C-H Bond Adjacent to Nitrogen of Tertiary Amides, Ureas, and Amines.

The article discusses radical hydroxyalkylation of carbon-hydrogen (C-H) bond adjacent to Nitrogen of tertiary amides, ureas and amines. The authors show that several tertiary amides, ureas, and amines undergo direct intermolecular addition to aldehydes under the EtB/air conditions, thereby providin...

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Publicado en:Journal of the American Chemical Society Vol. 127; no. 33; pp. 11610 - 11612
Autores principales: Yoshimitsu, Takehiko, Arano, Yoshimasa, Nagaoka, Hiroto
Formato: Artículo
Publicado: American Chemical Society 8/24/2005
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      dt: 8/24/2005
      vid: 127
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      pub: American Chemical Society
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        10.1021/ja053855q
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        atl: Radical Hydroxyalkylation of C-H Bond Adjacent to Nitrogen of Tertiary Amides, Ureas, and Amines.
      aug:
        au:
          Yoshimitsu, Takehiko
          Arano, Yoshimasa
          Nagaoka, Hiroto
        affil: Meiji Pharmaceutical University, 2-522-1 Noshio, Kiyose, Tokyo 204-8588, Japan.
      su:
        Chemical bonds
        Nitrogen
        Amides
        Urease
        Amines
        Aldehydes
      sug:
        subj:
          Chemical bonds
          Nitrogen
          Amides
          Urease
          Amines
          Aldehydes
      ab: The article discusses radical hydroxyalkylation of carbon-hydrogen (C-H) bond adjacent to Nitrogen of tertiary amides, ureas and amines. The authors show that several tertiary amides, ureas, and amines undergo direct intermolecular addition to aldehydes under the EtB/air conditions, thereby providing a unique and simple means for the radical sp C-H transformation of nitrogen-containing molecules. The amounts of C-H substrate and EtB influenced the efficiency of the reaction.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2005
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