Synthesis, thermodynamic and spectroscopic study of violurate salt.

The organic salts are a broad class of ionic chemicals with a variety of properties. Scientists have an interest in violurate salts because of their bright color and crystal structure. In this study, 4-chloroanilinium violurate salt was synthesized and identification using infrared spectroscopy, 13C...

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Publicado en:Journal of Basrah Researches (Sciences) Vol. 50; no. 1; pp. 203 - 214
Autores principales: Abdulzahra, Huda Nouri, H Ismael, Sadiq M., Almashal, Faeza Abdulkareem
Formato: Artículo
Publicado: Republic of Iraq Ministry of Higher Education & Scientific Research (MOHESR) 2024
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Acceso en línea:Ver este registro en EBSCOhost
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        atl: Synthesis, thermodynamic and spectroscopic study of violurate salt.
      aug:
        au:
          Abdulzahra, Huda Nouri
          H Ismael, Sadiq M.
          Almashal, Faeza Abdulkareem
        affil: Department of Chemistry, College of Education for pure sciences, University of Basrah, Basrah, Iraq.
      su:
        Chemical properties
        Density functional theory
        Infrared spectroscopy
        Nuclear magnetic resonance spectroscopy
        Crystal structure
      sug:
        subj:
          Chemical properties
          Density functional theory
          Infrared spectroscopy
          Nuclear magnetic resonance spectroscopy
          Crystal structure
      keyword:
        DFT
        hyperpolarizability
        polarizability
        violurate salt
        الاستقطابية
        املاح الفويلوريت
        فرط الاستقطابية
      ab: The organic salts are a broad class of ionic chemicals with a variety of properties. Scientists have an interest in violurate salts because of their bright color and crystal structure. In this study, 4-chloroanilinium violurate salt was synthesized and identification using infrared spectroscopy, 13C NMR spectroscopy and Electrospray ionization (ESI). Density functional theory (DFT) calculations have been performed using B3LYP/6-31++G**, and CAM-B3LYP/6-31++G** levels of theory. Practically, chloroanilinium ion (M+H) has a relative abundance of 100% in ESI+, indicating its excellent stability. The protonation formula for violuric acid (VA+H) shows instability, despite the observation of a low abundance of the (VA+3H) ion. DFT calculations demonstrate the exothermic nature of the salt formation reaction. The calculated enthalpy change is -26.861kJ in the B3LYP/6-31++G** level of theory and -31.82kJ in the CAM-B3LYP/6-31++G** level of theory.
      pubtype: Academic Journal
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      src: R
    language: English
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