Application of X-ray diffraction with Rietveld refinement to quantify mineral composition including crystalline silica in respirable dust.

This study aimed to test the use of Rietveld refinement on respirable aerosol samples to determine the phase of respirable crystalline silica (RCS) and other minerals. The results from the Rietveld refinement were compared to an external standard method and gravimetrical measurements. Laboratory sam...

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Published in:Journal of Occupational & Environmental Hygiene Vol. 22; no. 4; pp. 248 - 259
Main Authors: Halvorsen, Johanne Østereng, Stacey, Peter, Graff, Pål, Folven Gjengedal, Elin Lovise, Ervik, Torunn K.
Format: CEU research tables/charts Journal Article
Published: Taylor & Francis Ltd Apr2025
Online Access:View this record in EBSCOhost
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      jtl: Journal of Occupational & Environmental Hygiene
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      dt: Apr2025
      vid: 22
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      pub: Taylor & Francis Ltd
      place: Philadelphia, Pennsylvania
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        10.1080/15459624.2024.2443206
        184403097
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        atl: Application of X-ray diffraction with Rietveld refinement to quantify mineral composition including crystalline silica in respirable dust.
      aug:
        au:
          Halvorsen, Johanne Østereng
          Stacey, Peter
          Graff, Pål
          Folven Gjengedal, Elin Lovise
          Ervik, Torunn K.
        affil: STAMI, National Institute of Occupational Health, Oslo, Norway
      sug:
        subj:
          Dust Analysis
          Silicon Dioxide Analysis
          Air Pollutants, Occupational Analysis
          Minerals Analysis
          Environmental Monitoring Methods
          Human
          Regression
          Construction Materials
          Inhalation Exposure
          Occupational Exposure
          X-Rays
          Occupational Safety
          Occupational Health
          Wilcoxon Rank Sum Test
          Education, Continuing (Credit)
      ab: This study aimed to test the use of Rietveld refinement on respirable aerosol samples to determine the phase of respirable crystalline silica (RCS) and other minerals. The results from the Rietveld refinement were compared to an external standard method and gravimetrical measurements. Laboratory samples consisting of α-quartz, feldspar, and calcite with variable proportions and total mass loadings were made and analyzed using the NIOSH 7500 Silica, Crystalline, by XRD (filter redeposition) method, followed by Rietveld refinement. Field samples of respirable dust, from construction sites working with concrete, brick, and other materials were included. To correct for amorphous content and unidentified phases, an internal standard was added to the field samples, which were treated like laboratory samples. Rietveld refinement was successfully used for quantification of RCS in laboratory and field samples. The method showed comparable results to the NIOSH 7500 method for quartz and remained linear for laboratory samples up to 20 mg. The lowest quantified amounts of quartz in the laboratory samples were 5 µg. The two methods yielded similar results for RCS in field samples with a total mass of up to 15 mg and a quartz content of 1.8 wt% to 11 wt%. A total sample mass of above 0.5 mg was required for optimal quantification of crystalline phases by Rietveld refinement. The method proved useful in determining RCS and other crystalline components in field samples and corrected for interferences even with a complex matrix and high mass loading.
      pubtype: Academic Journal
      doctype:
        CEU
        research
        tables/charts
        Journal Article
      ougenre: Unknown
    language: English
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