Antibacterial effects and mechanisms of graphene oxide loaded on TiO2-nanotube-modified ti: an in vitro study.

Background: Peri-implant inflammation is an important factor affecting the success rate of dental implants. Improving the antibacterial performance of implants is an effective method to prevent and treat peri-implant inflammation. Methods: In this study, Graphene oxide (GO) was loaded onto Titanium...

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Publicado en:BMC Oral Health Vol. 25; no. 1; pp. 1 - 16
Autores principales: Wu, Keyi, Cao, Xu, Luo, Bin, Wang, Caiyun, Lu, Ran, Wang, Xin, Chen, Su
Formato: pictorial research tables/charts Journal Article
Publicado: BioMed Central 7/5/2025
Acceso en línea:Ver este registro en EBSCOhost
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        14726831
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      dt: 7/5/2025
      vid: 25
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      pub: BioMed Central
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        10.1186/s12903-025-06453-w
        186463881
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        atl: Antibacterial effects and mechanisms of graphene oxide loaded on TiO2-nanotube-modified ti: an in vitro study.
      aug:
        au:
          Wu, Keyi
          Cao, Xu
          Luo, Bin
          Wang, Caiyun
          Lu, Ran
          Wang, Xin
          Chen, Su
        affil: https://ror.org/013xs5b60 Laboratory of Biomaterials and Biomechanics, Beijing Key Laboratory of Tooth Regeneration and Function Reconstruction, Beijing Stomatological Hospital, Capital Medical University, 100050, Beijing, China
      sug:
        subj:
          Peri-Implantitis Drug Therapy
          Titanium Pharmacodynamics
          Antibiotics Pharmacodynamics
          Biocompatible Materials Pharmacodynamics
          Carbon Pharmacodynamics
          Materials Testing
          Nanostructures
          Titanium Analysis
          Gram-Negative Anaerobic Bacteria Drug Effects
          In Vitro Studies
          China
          Academic Medical Centers
          Microscopy
          Microscopy, Electron, Scanning
          Reactive Oxygen Species
          Spectrum Analysis, Raman
          Surface Properties
          X-Rays
          Cell Proliferation Drug Effects
          Fibroblasts Drug Effects
          Fluorescence Polarization Immunoassay
          Descriptive Statistics
          Data Analysis Software
          One-Way Analysis of Variance
          Oxidative Stress Drug Effects
          Funding Source
      ab: Background: Peri-implant inflammation is an important factor affecting the success rate of dental implants. Improving the antibacterial performance of implants is an effective method to prevent and treat peri-implant inflammation. Methods: In this study, Graphene oxide (GO) was loaded onto Titanium (Ti) dioxide nanotubes (TNT) to produce a material with good antibacterial effects and biocompatibility. TNT was prepared through anodization, and GO-loaded TNT-modified Ti (TNT-GO) was synthesized through electrodeposition. The materials were characterized using scanning electron microscopy (SEM), Raman spectroscopy, X-ray diffraction (XRD), and atomic force microscopy (AFM). Standard plate counting assay, methyl thiazolyl tetrazolium (MTT) assay, and fluorescence staining were used to assess the antibacterial effects of the samples. Bacterial morphology observations were conducted to explore the antibacterial mechanisms via SEM, transmission electron microscopy (TEM), reactive oxygen species (ROS) assay, and lactate dehydrogenase (LDH) cytotoxicity assay. Cell proliferation and morphological observations of the materials were performed to test the biocompatibility of TNT-GO. Results: The characteristic peaks of graphene oxide on TNT-GO were detected by Raman spectra. The results of contact angle test and AFM show that TNT-GO had the greatest hydrophilicity and the largest surface roughness. When P. gingivalis was cultured on the sample surfaces, the TNT-GO demonstrated the lowest bacterial adhesion, with significantly disrupted bacterial morphology. Specifically, the bacterial cells exhibited collapsed and ruptured cell membranes, leakage of intracellular contents, reduced membrane density, and phospholipid extraction. The TNT-GO group also showed the highest release of LDH extracellularly and the greatest ROS generation. The results of CCK-8 show that there was no significant difference between TNT-GO group and Ti group. The results of adherent cells morphology observation show that human gingival fibroblasts on TNT-GO group were in fusiformis and irregular triangle shapes while human gingival fibroblasts on TNT group and Ti group were in round shapes. Conclusions: The TNT-GO had good biocompatibility and a good antibacterial effect on Porphyromonas gingivalis. It can inhibit bacteria-derived soft tissue infections and bone resorption and may be a very promising implant material.
      pubtype: Academic Journal
      doctype:
        pictorial
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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