Design of All-Inorganic Molecular-Based Photocatalysts Sensitive to Visible Light: Ti(IV)—O—Ce(III) Bimetallic Assemblies on Mesoporous Silica.

The article reports on the first photocatalysis driven by the visible-light induced metal-to-metal charge transfer (MMCT) for hetero-bimettalic Ti(IV)-O—Ce(III) assemblies on the pore of mesoporous silica. The combination of Ti(IV) and Ce(III) enabled to drive the photocatalytic oxidative decomposit...

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Bibliographic Details
Published in:Journal of the American Chemical Society Vol. 129; no. 31; pp. 9596 - 9598
Main Authors: Nakamura, Ryuhei, Okamoto, Akihiro, Osawa, Hitoshi, Irie, Hiroshi, Hashimoto, Kazuhito
Format: Article
Published: American Chemical Society 8/8/2007
Subjects:
Online Access:View this record in EBSCOhost
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        10.1021/ja073668n
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        atl: Design of All-Inorganic Molecular-Based Photocatalysts Sensitive to Visible Light: Ti(IV)—O—Ce(III) Bimetallic Assemblies on Mesoporous Silica.
      aug:
        au:
          Nakamura, Ryuhei
          Okamoto, Akihiro
          Osawa, Hitoshi
          Irie, Hiroshi
          Hashimoto, Kazuhito
        affil:
          Department of Applied Chemistry, School of Engineering, University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan
          Japan Synchrotron Radiation Research Institute, 1-1-1, Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5198, Japan
          Exploratory Research for Advanced Technology (ERATO), JST
      su:
        Photocatalysis
        Charge transfer
        Ion exchange (Chemistry)
        Titanium
        Acetone
        Carbon dioxide
        Irradiation
      sug:
        subj:
          Photocatalysis
          Charge transfer
          Ion exchange (Chemistry)
          Titanium
          Acetone
          Carbon dioxide
          Irradiation
      ab: The article reports on the first photocatalysis driven by the visible-light induced metal-to-metal charge transfer (MMCT) for hetero-bimettalic Ti(IV)-O—Ce(III) assemblies on the pore of mesoporous silica. The combination of Ti(IV) and Ce(III) enabled to drive the photocatalytic oxidative decomposition of 2-propanol into acetone and carbon dioxide under visible-light irradiation. Results of the study and its implications are presented and discussed.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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