Immunomagnetic Diffractometry for Detection of Diagnostic Serum Markers.

We describe an integrated approach for detection of diagnostic markers using in situ assembled optical diffraction gratings in combination with immunomagnetic capture. Folate receptor (FR), a serum protein indicative of various cancers, was chosen as a model system to demonstrate the potential of th...

Descripción completa

Detalles Bibliográficos
Publicado en:Journal of the American Chemical Society Vol. 129; no. 51; pp. 15824 - 15830
Autores principales: Acharya, Ghanashyam, Chun-Li Chang, Doorneweerd, Derek D., VIashi, Erina, Henne, Walter A., Hartmann, Lynn C., Low, Philip S., Savran, Cagri A.
Formato: Artículo
Publicado: American Chemical Society 12/26/2007
Materias:
Acceso en línea:Ver este registro en EBSCOhost
fields @attributes:
  recordID: 1
pdfLink:
plink: https://search.ebscohost.com/login.aspx?direct=true&db=hlh&AN=28843167&site=ehost-live
header:
  @attributes:
    shortDbName: hlh
    uiTerm: 28843167
    longDbName: Humanities International Complete
    uiTag: AN
  controlInfo:
    bkinfo:
    jinfo:
      jid:
        00027863
        ACS
      jtl: Journal of the American Chemical Society
      issn: 00027863
      maglogo: N
    pubinfo:
      dt: 12/26/2007
      vid: 129
      iid: 51
      pid: 997
      pub: American Chemical Society
    artinfo:
      ui:
        28843167
        10.1021/ja073094m
      ppf: 15824
      ppct: 6
      formats:
      tig:
        atl: Immunomagnetic Diffractometry for Detection of Diagnostic Serum Markers.
      aug:
        au:
          Acharya, Ghanashyam
          Chun-Li Chang
          Doorneweerd, Derek D.
          VIashi, Erina
          Henne, Walter A.
          Hartmann, Lynn C.
          Low, Philip S.
          Savran, Cagri A.
        affil:
          Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907
          School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907
          Department of Chemistry, Purdue University, West Lafayette, Indiana 47907
          Department of Oncology, Mayo Clinic, Rochester, Minnesota 55905
          School of Mechanical Engineering, Purdue University, West Lafayette, Indiana 47907
          Weldon School of Biomedical Engineering, Purdue University, West Lafayette, Indiana 47907
      su:
        Optical diffraction
        Vitamin B complex
        Blood proteins
        Cancer diagnosis
        Immunoglobulins
        Physical & theoretical chemistry
      sug:
        subj:
          Optical diffraction
          Vitamin B complex
          Blood proteins
          Cancer diagnosis
          Immunoglobulins
          Physical & theoretical chemistry
      ab: We describe an integrated approach for detection of diagnostic markers using in situ assembled optical diffraction gratings in combination with immunomagnetic capture. Folate receptor (FR), a serum protein indicative of various cancers, was chosen as a model system to demonstrate the potential of the method. Magnetic beads coupled to FR antibody were used to capture FR from serum. The FR-bound magnetic beads self-assembled onto microcontact-printed folate-coupled BSA (F-BSA) patterns to form diffraction gratings which served to detect FR by measuring the diffraction intensities caused by laser illumination. The FR-containing beads, upon binding to the F-BSA surface, served as intrinsic signal enhancement agents, circumventing the need for additional enzymatic signal amplification or fluorescent labeling steps. With this approach, a detection sensitivity of 700 fM (20 pg/mL) was achieved. The potential use of this approach in clinical diagnostics was demonstrated by measuring FR concentration in blood samples obtained from cancer patients.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
    refInfo:
    copyright:
      @attributes:
        flag: Y
      dt:
        @attributes:
          year: 2007
    holdings:
      @attributes:
        islocal: N