A Path Sampling Study of Ru-Hydride-Catalyzed H Hydrogenation of Ethylene.

The article reports on a molecular dynamics and path sampling study of a catalytic cycle to resolve the nature of a ruthenium dihydride intermediate for ethylene dehydrogenation. The ethylene insertion process using path sampling were harvested. The trajectories provide a range of vibrational energy...

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Bibliographic Details
Published in:Journal of the American Chemical Society Vol. 130; no. 23; pp. 7218 - 7220
Main Authors: Rowley, Christopher N., Woo, Tom K.
Format: Article
Published: American Chemical Society 6/11/2008
Subjects:
Online Access:View this record in EBSCOhost
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        10.1021/ja802219a
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        atl: A Path Sampling Study of Ru-Hydride-Catalyzed H Hydrogenation of Ethylene.
      aug:
        au:
          Rowley, Christopher N.
          Woo, Tom K.
        affil: Centre for Catalysis Research and Innovation, Department of Chemistry, University of Ottawa, /0 Marie-Curie, Ottawa, ON, KIN 6N5 Canada
      su:
        Molecular dynamics
        Sampling (Process)
        Ethylene
        Dehydrogenation
        Elimination reactions
        Spectral energy distribution
      sug:
        subj:
          Molecular dynamics
          Sampling (Process)
          Ethylene
          Dehydrogenation
          Elimination reactions
          Spectral energy distribution
      ab: The article reports on a molecular dynamics and path sampling study of a catalytic cycle to resolve the nature of a ruthenium dihydride intermediate for ethylene dehydrogenation. The ethylene insertion process using path sampling were harvested. The trajectories provide a range of vibrational energy distributions which reflect the localization of kinetic energy.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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