Heavier Group 2 Metals and Intermolecular Hydroamination: A Computational and Synthetic Assessment.

The article presents a study which offers a computational and synthetic assessment of heavier group 2 metals and intermolecular hydroamination. The study utilized a density functional theory (DFT) that aims to highlight the intrinsic reaction barriers in the catalytic mechanism. The results of the s...

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Publicado en:Journal of the American Chemical Society Vol. 131; no. 36; pp. 12906 - 12908
Autores principales: Barrett, Anthony G. M., Brinkmann, Christine, Crimmin, Mark R., Hill, Michael S., Hunt, Patricia, Procopiou, Panayiotis A.
Formato: Artículo
Publicado: American Chemical Society 9/16/2009
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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        atl: Heavier Group 2 Metals and Intermolecular Hydroamination: A Computational and Synthetic Assessment.
      aug:
        au:
          Barrett, Anthony G. M.
          Brinkmann, Christine
          Crimmin, Mark R.
          Hill, Michael S.
          Hunt, Patricia
          Procopiou, Panayiotis A.
        affil:
          Department of Chemistry, Imperial College London, Exhibition Road, South Kensington, London SW7 2AZ, U.K.
          Department of Chemistry, University of Bath, Claverton Down, Bath BA2 7AY, U.K.
          GlaxoSmithKline Medicines Research Centre, Gunnels Wood Road, Stevenage, Hertfordshire SG1 2NY, U.K.
      su:
        Metals
        Density functionals
        Functional analysis
        Catalysis
        Alkenes
        Coulomb functions
        Chemical research
        Inorganic chemistry
      sug:
        subj:
          Metals
          Density functionals
          Functional analysis
          Catalysis
          Alkenes
          Coulomb functions
          Chemical research
          Inorganic chemistry
      ab: The article presents a study which offers a computational and synthetic assessment of heavier group 2 metals and intermolecular hydroamination. The study utilized a density functional theory (DFT) that aims to highlight the intrinsic reaction barriers in the catalytic mechanism. The results of the study support rate-determining alkene insertion that occurred inside a catalytic cycle dominated by Coulomb interactions.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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