Magnetochromatic Microspheres: Rotating Photonic Crystals.

Magnetochromatic microspheres have been fabricated through instant assembly of superparamagnetic (SPM) colloidal particles inside emulsion droplets of UV curable resin followed by an immediate UV curing process to polymerize the droplets and fix the ordered structures. When dispersed in the liquid d...

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Publicado en:Journal of the American Chemical Society Vol. 131; no. 43; pp. 15687 - 15695
Autores principales: Jianping Ge, Howon Lee, Le He, Junhoi Kim, Zhenda Lu, Hyoki Kim, Goebl, James, Sunghoon Kwon, Yadong Yin
Formato: Artículo
Publicado: American Chemical Society 11/4/2009
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      dt: 11/4/2009
      vid: 131
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      pub: American Chemical Society
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        10.1021/ja903626h
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        atl: Magnetochromatic Microspheres: Rotating Photonic Crystals.
      aug:
        au:
          Jianping Ge
          Howon Lee
          Le He
          Junhoi Kim
          Zhenda Lu
          Hyoki Kim
          Goebl, James
          Sunghoon Kwon
          Yadong Yin
        affil:
          Department of Chemistry, University of California, Riverside, California 92521
          School of Electrical Engineering and Computer Science, Seoul National University, San 56-1, Shillim 9-dong, Gwanak-ku, Seoul 151- 744, South Korea
      su:
        Photonics
        Optical diffraction
        Polymerization
        Magnetic fields
        Colloidal crystals
        Emulsions
      sug:
        subj:
          Photonics
          Optical diffraction
          Polymerization
          Magnetic fields
          Colloidal crystals
          Emulsions
      ab: Magnetochromatic microspheres have been fabricated through instant assembly of superparamagnetic (SPM) colloidal particles inside emulsion droplets of UV curable resin followed by an immediate UV curing process to polymerize the droplets and fix the ordered structures. When dispersed in the liquid droplets, superparamagnetic FeO@SiO core/shell particles self-organize under the balanced interaction of repulsive and attractive forces to form one-dimensional chains, each of which contains periodically arranged particles diffracting visible light and displaying field-tunable colors. UV initiated polymerization of the oligomers of the resin fixes the periodic structures inside the droplet microspheres and retains the diffraction property. Because the superparamagnetic chains tend to align themselves along the field direction, it is very convenient to control the orientation of such photonic microspheres and, accordingly, their diffractive colors, by changing the orientation of the crystal lattice relative to the incident light using magnetic fields. The excellent stability together with the capability of fast on/off switching of the diffraction by magnetic fields makes the system suitable for applications such as color display, rewritable signage, and sensors. As a simple demonstration, we have fabricated a display unit that has on/off bistable states by embedding the magnetochromatic microspheres in a matrix that can thermally switch between solid and liquid phases.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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