An Unusual Hydrogen Migration/C--H Activation Reaction with Group 3 Metals.

A novel hydrogen migration from the phenyl ring to the pyridine ring of an yttrium pyridyl complex supported by a 1,1′-ferrocene diamide ligand is reported. Density functional theory calculations were instrumental in probing the mechanism for this transformation.

Detalles Bibliográficos
Publicado en:Journal of the American Chemical Society Vol. 133; no. 13; pp. 4680 - 4684
Autores principales: Williams, Bryan N., Benitez, Diego, Miller, Kevin L., Tkatchouk, Ekaterina, Goddard, III, William A., Diaconescu, Paula L.
Formato: Artículo
Publicado: American Chemical Society 4/6/2011
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      dt: 4/6/2011
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        10.1021/ja110505r
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        atl: An Unusual Hydrogen Migration/C--H Activation Reaction with Group 3 Metals.
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          Williams, Bryan N.
          Benitez, Diego
          Miller, Kevin L.
          Tkatchouk, Ekaterina
          Goddard, III, William A.
          Diaconescu, Paula L.
        affil:
          Department of Chemistry & Biochemistry, University of California, Los Angeles, California 90095, United States
          Materials and Process Simulation Center, California Institute of Technology, Pasadena, California 91125, United States
      su:
        Phenyl compounds
        Pyridine
        Ferrocene
        Density functionals
        Biochemical mechanism of action
      sug:
        subj:
          Phenyl compounds
          Pyridine
          Ferrocene
          Density functionals
          Biochemical mechanism of action
      ab: A novel hydrogen migration from the phenyl ring to the pyridine ring of an yttrium pyridyl complex supported by a 1,1′-ferrocene diamide ligand is reported. Density functional theory calculations were instrumental in probing the mechanism for this transformation.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2011
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