Coherent Transport through Spin-Crossover Single Molecules.

Coherent quantum transport calculations were performed for high- and low-spin states of a mononuclear Fe complex showing spin-crossover behavior using density functional theory methods combined with the non-equilibrium Green functions procedure. The high-spin state has a larger conductivity than the...

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Publicado en:Journal of the American Chemical Society Vol. 134; no. 2; pp. 777 - 780
Autores principales: Aravena, Daniel, Ruiz, Eliseo
Formato: Artículo
Publicado: American Chemical Society 1/18/2012
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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      pub: American Chemical Society
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        atl: Coherent Transport through Spin-Crossover Single Molecules.
      aug:
        au:
          Aravena, Daniel
          Ruiz, Eliseo
        affil: Departament de Química Inorgànica and Institut de Recerca de Química Teòrica i Computacional, Universitat de Barcelona, Diagonal 645, Barcelona E-08028, Spain
      su:
        Molecular rotation
        Inorganic chemistry
        Density functionals
        Green's functions
        Nuclear spin
        Metal complexes
        Iron
      sug:
        subj:
          Molecular rotation
          Inorganic chemistry
          Density functionals
          Green's functions
          Nuclear spin
          Metal complexes
          Iron
      ab: Coherent quantum transport calculations were performed for high- and low-spin states of a mononuclear Fe complex showing spin-crossover behavior using density functional theory methods combined with the non-equilibrium Green functions procedure. The high-spin state has a larger conductivity than the low-spin state; furthermore, it behaves as a spin filter, giving a β-polarized current.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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          year: 2012
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