Theoretical Study of Reactivity of Ge(II)-hydride Compound: Comparison with Rh(I)-Hydride Complex and Prediction of Full Catalytic Cycle by Ge(II)-hydride.

The reaction of a Ge(II) hydride compound HC{CMeArN}GeH (Ar = 2,6-iPrCH) 1 with 2,2,2-trifluoroacetophenone (CFPhCO) is theoretically investigated with density functional theory and spin-component-scaled second-order Møller–Plesset methods. This reaction easily occurs with moderate activation barrie...

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Publicado en:Journal of the American Chemical Society Vol. 135; no. 24; pp. 8955 - 8966
Autores principales: Nozomi Takagi, Shigeyoshi Sakaki
Formato: Artículo
Publicado: American Chemical Society 6/19/2013
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Acceso en línea:Ver este registro en EBSCOhost