Assessment of urinary mephenytoin metrics to phenotype for CYP2C19 and CYP2B6 activity.

OBJECTIVES: (S)-Mephenytoin is selectively metabolised to (S)-4'-hydroxymephenytoin by CYP2C19. The urinary excretion of 4'-hydroxymephenytoin reflects the activity of individual enzymes. We evaluated fractioned urinary collection and beta-glucuronidase pre-treatment in order to determine the optima...

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Publicado en:European Journal of Clinical Pharmacology Vol. 64; no. 4; pp. 387 - 399
Autores principales: Klaassen T, Jetter A, Tomalik-Scharte D, Kasel D, Kirchheiner J, Jaehde U, Fuhr U
Formato: equations & formulas research tables/charts Journal Article
Publicado: Springer Nature Apr2008
Acceso en línea:Ver este registro en EBSCOhost
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      dt: Apr2008
      vid: 64
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      pub: Springer Nature
      place: New York, New York
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        10.1007/s00228-007-0416-z
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        atl: Assessment of urinary mephenytoin metrics to phenotype for CYP2C19 and CYP2B6 activity.
      aug:
        au:
          Klaassen T
          Jetter A
          Tomalik-Scharte D
          Kasel D
          Kirchheiner J
          Jaehde U
          Fuhr U
        affil: Department of Pharmacology, Clinical Pharmacology, Hospital of the University of Cologne, Gleueler Str. 24, 50931 Köln, Germany.
      sug:
        subj:
          Enzymes Physiology
          Phenotype
          Phenytoin Urine
          Descriptive Statistics
          Male
          Urinalysis Methods
          White Persons
          Human
          Male
      ab: OBJECTIVES: (S)-Mephenytoin is selectively metabolised to (S)-4'-hydroxymephenytoin by CYP2C19. The urinary excretion of 4'-hydroxymephenytoin reflects the activity of individual enzymes. We evaluated fractioned urinary collection and beta-glucuronidase pre-treatment in order to determine the optimal CYP2C19 metrics. We also assessed whether urinary excretion of N-desmethylmephenytoin (nirvanol) might be a useful CYP2B6 metric in in vivo studies. METHODS: A 50-mg dose of mephenytoin was administered to 52 volunteers as a component of phenotyping cocktails in four separate studies. Urine was collected up to 166 h post-dose. Urinary excretion of 4'-hydroxymephenytoin and nirvanol was quantified by liquid chromatography-tandem mass spectrometry, and common CYP2C19 and CYP2B6 genotypes were determined. RESULTS: Cumulative excretion of 4'-hydroxymephenytoin in urine with beta-glucuronidase treatment collected from before mephenytoin administration up to 12-16 h thereafter showed the greatest difference between CYP2C19 genotypes and the lowest intra-individual variability (7%). Renal elimination of nirvanol was highest for a *4/*4 individual and lowest for individuals carrying the *5/*5 and *1/*7 genotype, but lasted for several weeks, thus making its use in cross-over studies difficult. CONCLUSION: Cumulative urinary excretion of 4'-hydroxymephenytoin 0-12 h post-administration is a sensitive and reproducible metric of CYP2C19 activity, enabling the effect of a drug on CYP2C19 to be assessed in a small sample size of n = 6 volunteers. While nirvanol excretion may reflect CYP2B6 activity in vivo, it is not useful for CYP2B6 phenotyping.
      pubtype: Academic Journal
      doctype:
        equations & formulas
        research
        tables/charts
        Journal Article
      ougenre: Article
    language: English
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