Conjugation to a cell-penetrating peptide drives the tumour accumulation of the GLP1R antagonist exendin(9-39).

Purpose: Exendin, an analogue of the glucagon-like peptide 1 (GLP1), is an excellent tracer for molecular imaging of pancreatic beta cells and beta cell-derived tumours. The commonly used form, exendin-4, activates the GLP1 receptor and causes internalisation of the peptide-receptor complex. As a co...

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Published in:European Journal of Nuclear Medicine & Molecular Imaging Vol. 50; no. 4; pp. 996 - 1005
Main Authors: Collado Camps, Estel, van Lith, Sanne A. M., Kip, Annemarie, Frielink, Cathelijne, Joosten, Lieke, Brock, Roland, Gotthardt, Martin
Format: Journal Article
Published: Springer Nature Mar2023
Online Access:View this record in EBSCOhost
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      dt: Mar2023
      vid: 50
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      pub: Springer Nature
      place: New York, New York
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        10.1007/s00259-022-06041-y
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        atl: Conjugation to a cell-penetrating peptide drives the tumour accumulation of the GLP1R antagonist exendin(9-39).
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        au:
          Collado Camps, Estel
          van Lith, Sanne A. M.
          Kip, Annemarie
          Frielink, Cathelijne
          Joosten, Lieke
          Brock, Roland
          Gotthardt, Martin
        affil: Department of Medical Imaging, Radboudumc, P.O. Box 9101, 6500 HB, Nijmegen, The Netherlands
      sug:
      ab: Purpose: Exendin, an analogue of the glucagon-like peptide 1 (GLP1), is an excellent tracer for molecular imaging of pancreatic beta cells and beta cell-derived tumours. The commonly used form, exendin-4, activates the GLP1 receptor and causes internalisation of the peptide-receptor complex. As a consequence, injection of exendin-4 can lead to adverse effects such as nausea, vomiting and hypoglycaemia and thus requires close monitoring during application. By comparison, the antagonist exendin(9-39) does not activate the receptor, but its lack of internalisation has precluded its use as a tracer. Improving the cellular uptake of exendin(9-39) could turn it into a useful alternative tracer with less side-effects than exendin-4. Methods: We conjugated exendin-4 and exendin(9-39) to the well-known cell-penetrating peptide (CPP) penetratin. We evaluated cell binding and internalisation of the radiolabelled peptides in vitro and their biodistribution in vivo. Results: Exendin-4 showed internalisation irrespective of the presence of the CPP, whereas for exendin(9-39) only the penetratin conjugate internalised. Conjugation to the CPP also enhanced the in vivo tumour uptake and retention of exendin(9-39). Conclusion: We demonstrate that penetratin robustly improves internalisation and tumour retention of exendin(9-39), opening new avenues for antagonist-based in vivo imaging of GLP1R.
      pubtype: Academic Journal
      doctype: Journal Article
      ougenre: Article
    language: English
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