A New Class of Mixed-Valence Systems with Orbitally Degenerate Organic Redox Centers. Examples Based on Hexa-Rhenium Molecular Prisms.

The article presents information on mixed-valence (MV) systems with orbitally degenerate organic redox centers. The most common examples of MV systems are of the type Mn-bridge, where M is a transition metal and the bridge is an organic linker. The excited-state calculations carried out for a nearly...

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Publicado en:Journal of the American Chemical Society Vol. 128; no. 39; pp. 12592 - 12594
Autores principales: Dinolfo, Peter H., Coropceanu, Veaceslav, Brédas, Jean-Luc, Hupp, Joseph T.
Formato: Artículo
Publicado: American Chemical Society 10/4/2006
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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        atl: A New Class of Mixed-Valence Systems with Orbitally Degenerate Organic Redox Centers. Examples Based on Hexa-Rhenium Molecular Prisms.
      aug:
        au:
          Dinolfo, Peter H.
          Coropceanu, Veaceslav
          Brédas, Jean-Luc
          Hupp, Joseph T.
        affil:
          Department of Chemistry, Stanford University, Stanford, CA 94306.
          School of Chemistry and Biochemistry, Georgia Institute of Technology, Atlanta, Georgia 30332.
          Department of Chemistry, Northwestern University, Evanston, Illinois 60208.
      su:
        Valence fluctuations
        Oxidation-reduction reaction
        Transition metals
        Linkers (Computer programs)
      sug:
        subj:
          Valence fluctuations
          Oxidation-reduction reaction
          Transition metals
          Linkers (Computer programs)
      ab: The article presents information on mixed-valence (MV) systems with orbitally degenerate organic redox centers. The most common examples of MV systems are of the type Mn-bridge, where M is a transition metal and the bridge is an organic linker. The excited-state calculations carried out for a nearly trigonal symmetry of the model system indicate some build up of IT character and an increase in intensity for other transitions.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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