Directly Pd(II)-Bridged Porphyrin Belts with Remarkable Curvatures.

A β,β'-doubly 2,6-pyridylene-bridged porphyrin dimer and trimer were prepared by Suzuki-Miyaura coupling reactions and confirmed to have largely bent structures. These oligopor- phyrins were readily metalated via meso-C-H bond activation with the assistance of the pyridyl nitrogen atoms to produce t...

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Publicado en:Journal of the American Chemical Society Vol. 132; no. 34; pp. 11868 - 11870
Autores principales: Jianxin Song, Aratani, Naoki, Ji Haeng Heo, Dongho Kim, Shinokubo, Hiroshi, Osuka, Atsuhiro
Formato: Artículo
Publicado: American Chemical Society 9/1/2010
Materias:
Acceso en línea:Ver este registro en EBSCOhost
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        10.1021/ja1046654
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        atl: Directly Pd(II)-Bridged Porphyrin Belts with Remarkable Curvatures.
      aug:
        au:
          Jianxin Song
          Aratani, Naoki
          Ji Haeng Heo
          Dongho Kim
          Shinokubo, Hiroshi
          Osuka, Atsuhiro
        affil:
          Department of Chemistry, Graduate School of Science, Kyoto University, Sakyo-ku, Kyoto 606-8502, Japan
          PRESTO, Japan Science and Technology Agency, Spectroscopy Laboratory for Functional π-Electronic Systems, Seoul 120-749, Korea
          Department of Chemistry, Yonsei University, Seoul 120-749, Korea
          Department of Applied Chemistry, Graduate School of Engineering, Nagoya University, Chikusa-ku, Nagoya 463-8603, Japan
      su:
        Porphyrins
        Hydrogen bonding
        Palladium
        Nitrogen
        Optical diffraction
        Ultraviolet radiation
      sug:
        subj:
          Porphyrins
          Hydrogen bonding
          Palladium
          Nitrogen
          Optical diffraction
          Ultraviolet radiation
      ab: A β,β'-doubly 2,6-pyridylene-bridged porphyrin dimer and trimer were prepared by Suzuki-Miyaura coupling reactions and confirmed to have largely bent structures. These oligopor- phyrins were readily metalated via meso-C-H bond activation with the assistance of the pyridyl nitrogen atoms to produce the corresponding Pd(II) complexes, which display even larger bent structures and larger TPA values at 800 nm.
      pubtype: Academic Journal
      doctype: Article
      src: R
    language: English
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